Download Crosslinking and Scission in Polymers by A. Charlesby (auth.), O. Güven (eds.) PDF

By A. Charlesby (auth.), O. Güven (eds.)

MOLECULAR WEIGHr alterations AND NE1WORK FORMATION through SCISSION AND CROSSUNKING A. Charlesby 1 creation major Chain Scission of Polymers ____________________________ _ ________________________ _ 1 Crosslinking ______ . . . . . . . . . . . . . . . . . . . . . . _ . . . . . . . _ . . . . . . . . . . . . . . . . _ . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . __ . . . . _ . . . . . . . . . . . _ . . . . . . . . ___ . . _. __ . . . . _. _. _____ . _____ . _ four five Random Crosslinking . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . _ . . . . . . . _ . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . more advantageous Crosslinking . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . eight different kinds of Crosslinking . . . . . . . . . . . . . _ . . . . . . . . . . . . . . . . . _ . . . . . . . . . . . . . . . _ . . . . . . . . . . . . . . . . _. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 10 mixed Crosslinking and Scission ___________ _________________ ______ _ ______________ . _. _. eleven Antioxidants . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . eleven Fillers . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . _ . . . . . . . . . . __ . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . _ . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . __ . . . 12 Crosslinking of Polymers in answer ________________________________ . . ______________ . . . . __ 12 References _. __ _ thirteen excessive strength RADIATION-AND UV UGHr-INDUCED CROSSLINKING AND CHAIN SCISSION w. Schnabel advent 15 significance of Radiation-Induced Crosslinking and Main-Chain Scission in Linear Polymers ___________________________ _________________ 15 different types of Radiation and Radiation resources _. ___________________________ . . . . . . . . . _ . . . . . . _ . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . _ . . . . . . . . . . _. _. _ . . __ . . . sixteen Absorption of Radiation . . _ . . . . _ . . . . . . _ . . _ . . __ . _ . . . . . . . . ____ . . . _ . . . . . . . . . . . . __ . . . . _ . . . . . . . . . _ . . . . _ . . . . . . _ . . . _ . . _ . . . . . . . . . . . . . . . . . . . . . _ . . . . . __ . . . . . . . . . . . _ . . . . . _____ . . . . . . . . . ___ . . . sixteen basic points pertaining to XL and CS in Linear Polymers ______________________ . _________ . _____ . _____ 22 Random and particular website assaults . . . . . . . _. ____ . _ . . . _ . . . . . . . . . . __ . . . . . . . . . . . . . _ . . ___ . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . _ . . . . . _ . . . . . __ . . . . _ . . . . . . _ . . . . __ . ___ . . . . . . . . . . __ . . _ 22 Detection of XL and CS . . . _. _ . . . . . . . . . . . . . . . _. __ . . . _ . . . . . . . . . . . . ___ . . . . . . . __ . . . _ . . . _ . . . . . . . . ____ . . . . . . . . . . . . . . . . . . _ . . . . _ . . . . . _ . . . . . . . . . . . . . . . . . . . . __ . . . . . _ . . . . _ . . . . . _. _ . . . . _ . . . . . . . 22 Simultaneous XL and CS Mechanisms 25 Ion Beam-Induced Radiation results In Linear Polymers ____________________________________________________ .

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6 Sotobayashi et al. 4 Klaumlinzer, Schnabel (1988) 0 0 Table 3 shows that G(S) decreases with increasing stopping power. Notably, in the case of PSt the 100 eV yield of crosslinking was found to be almost independent of LET. This can be seen from Table 4. Table 4. 05 O'Donnell et al. 03 Klaumlinzer, Schnabel (1988)! l, 8+ 18. 85 MeV//Lm. 37 MeV//Lm both for 275 MeV and 200 keY neon ions and that, therefore, the differences in G(X) found by the two groups could reflect a strong track structure effect, as discussed before.

L, 8+ 18. 85 MeV//Lm. 37 MeV//Lm both for 275 MeV and 200 keY neon ions and that, therefore, the differences in G(X) found by the two groups could reflect a strong track structure effect, as discussed before. A strong dependence of 32 G(X) on E was also reported recently by Aoki et al. (1988) for the irradiation of PSt with H+ and He+ ions. Also these authors interpret their results partly on the basis of a track structure effect. Actually, the beam intensity in the experiments with ions of relatively low energy was very high.

Biol. Chem. ;aturforsch. J. Sc. Sci. Ed. Chem. Photochem. Stabil. 8. Naturforsch. Schnabel (1975), Macromolecules 8, 430 H. Polym. J. Naturforsch. Biophys. Ed. Biol. J. Chem. Schnabel (1986), Racliat. Chem. Naturforsch. Schulte-Frohlinde (1978). ), Springer-Verlag, Berlin, p. 204 C. Phys. Chem. Schnabel (1983), Makromo 1. Chem. , Rapid. Naturforsch. Chem. Biol. Chem. urforsch. Biol.

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